Friday, January 11, 2013

1301.2168 (Gavin D. Scott et al.)

Transport Characterization of Kondo-Correlated Single Molecule Devices    [PDF]

Gavin D. Scott, Douglas Natelson, Stefan Kirchner, Enrique Muñoz
A single molecule break junction device serves as a tunable model system for probing the many body Kondo state. The low-energy properties of this state are commonly described in terms of a Kondo model, where the response of the system to different perturbations is characterized by a single emergent energy scale, $k_B{T_K}$. Comparisons between different experimental systems have shown issues with numerical consistency. With a new constrained analysis examining the dependence of conductance on temperature, bias, and magnetic field simultaneously, we show that these deviations can be resolved by properly accounting for background, non-Kondo contributions to the conductance that are often neglected. We clearly demonstrate the importance of these non-Kondo conduction channels by examining transport in devices with total conductances exceeding the theoretical maximum due to Kondo-assisted tunneling alone.
View original: http://arxiv.org/abs/1301.2168

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